Nature research paper: Synthesis and target annotation of the alkaloid GB18
. Limited, variable supply of GB alkaloids. Here we report a solution to the supply of GB18, a structural outlier and putative psychotropic principle ofbark.
Efficient access to its challenging tetrahedral attached-ring motif required the development of a ligand-controlled-selective cross-electrophile coupling and a diastereoselective hydrogenation of a rotationally-dynamic pyridine.
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